RELEASE_NOTES 12 September 2003 The major changes and new features of this release are: 1) Modified the treatment of secondary organic aerosol (SOA) formation + The SOA algorithm has been modified to make the gas-particle partitioning of semi-volatiles reversible + Eliminated SOA production from anthropogenic alkenes + Adjusted yields of semi-volatiles from alkanes and aromatics to account for emissions of non-SOA producers being lumped with those from SOA-producers + Modified gas-phase monoterpene reactions rates in RADM2 and CB4 2) Modified the heterogeneous N2O5 reaction probability 3) Added an Euler Backward Iterative (EBI) gas-phase chemistry solver for the CB4 family of chemical mechanism 4) Implemented layer-dependent horizontal advection time-stepping 5) Changed the order of the time splitting science processes: Previous order New order -------------------- -------------------- advection +----> vertical diffusion mass-adjustment | advection horizontal diffusion | mass-adjustment vertical diffusion ----+ horizontal diffusion clouds clouds chemistry chemistry aerosols aerosols 6) Updated all gas-phase chemical mechanisms (cb4, radm2, saprc) + New deposition velocity surrogates + New cloud scavenging surrogates + Zeroed reaction rate constant for N2O5 + H2O -> 2HNO3 in all /aero3 mechanisms + Changed names of aero3/SOA NR species + For CB4, eliminated advection and diffusion of fast-reacting species 7) Cloud enhancements/updates + Modified to use effective Henry's Law constant for scavenging + Updated and added new coefficients to the Henry's Law constant table + Revised the timestep calculation in the aqueous chemistry subroutine + Updated the coarse-mode aerosol number washout 8) Other enhancements and bug fixes + Changed the units for aerosol for vertical diffusion to molar mixing ratio instead of mass density concentration + Updated the minimum aerosol concentration array and bug fix in coarse-mode aerosol standard deviation in the aerosol dry deposition subroutine + Added compatibility with emissions files that contain PM10 and speciated PM2.5 but do not contain PMC + Removed unused SUBST_GRID_ID + Fixed index bug in load_cgrid + Bug fix for no gas emissions species + Fixed NFS latency problems for parallel runs on an MPICH cluster